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J Am Chem Soc. 2002 Jul 31;124(30):8812-3.

High-performance, solution-processed organic thin film transistors from a novel pentacene precursor.

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1
IBM Research Division, T. J. Watson Research Center, Yorktown Heights, New York 10598, USA. afzali@us.ibm.com

Abstract

The Lewis acid-catalyzed Diels-Alder reaction of the organic semiconductor pentacene with N-sulfinylacetamide yields a soluble adduct. Spin-coated thin films of this adduct undergo solid-phase conversion to form thin films of pentacene at moderate temperatures. Organic thin film transistors fabricated by spin-coating this adduct, followed by thermal conversion to pentacene, exhibit the highest mobility reported to date for a solution-processed organic semiconductor.

PMID:
12137531
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