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Strong Ferromagnetic Exchange Coupling and Single-Molecule Magnetism in MoS43--Bridged Dilanthanide Complexes.
Darago LE, Boshart MD, Nguyen BD, Perlt E, Ziller JW, Lukens WW, Furche F, Evans WJ, Long JR. Darago LE, et al. J Am Chem Soc. 2021 Jun 9;143(22):8465-8475. doi: 10.1021/jacs.1c03098. Epub 2021 May 24. J Am Chem Soc. 2021. PMID: 34029482
UV-Vis-NIR diffuse reflectance spectra and DFT calculations of 1-Ln reveal a low-energy metal-to-metal charge transfer transition assigned to charge transfer from the singly occupied 4d(z(2)) orbital of Mo(V) to the empty 5d orbitals of the lanthanides (4d in the case of 1 …
UV-Vis-NIR diffuse reflectance spectra and DFT calculations of 1-Ln reveal a low-energy metal-to-metal charge transfer transition assigned t …
Synthesis, Structure, and Magnetism of Tris(amide) [Ln{N(SiMe3 )2 }3 ]1- Complexes of the Non-traditional +2 Lanthanide Ions.
Ryan AJ, Darago LE, Balasubramani SG, Chen GP, Ziller JW, Furche F, Long JR, Evans WJ. Ryan AJ, et al. Chemistry. 2018 May 28;24(30):7702-7709. doi: 10.1002/chem.201800610. Epub 2018 May 3. Chemistry. 2018. PMID: 29490123
Crystallographic data as well as UV/Vis, magnetic susceptibility, and density functional theory studies are consistent with the accessibility of 4f(n) 5d(1) configurations for Ln(2+) ions in this tris(silylamide) ligand environment. ...
Crystallographic data as well as UV/Vis, magnetic susceptibility, and density functional theory studies are consistent with the accessibilit …
Utility of Lithium in Rare-Earth Metal Reduction Reactions to Form Nontraditional Ln2+ Complexes and Unusual [Li(2.2.2-cryptand)]1+ Cations.
Huh DN, Darago LE, Ziller JW, Evans WJ. Huh DN, et al. Inorg Chem. 2018 Feb 19;57(4):2096-2102. doi: 10.1021/acs.inorgchem.7b03000. Epub 2018 Feb 2. Inorg Chem. 2018. PMID: 29393645
Magnetic susceptibility data on these new examples of nontraditional divalent lanthanide complexes are consistent with 4f(n)5d(1) electronic configurations. The Dy and Ho complexes have exceptionally high single-ion magnetic moments, 11.35 and 11.67 mu(B), respectively. .. …
Magnetic susceptibility data on these new examples of nontraditional divalent lanthanide complexes are consistent with 4f(n)5d(1) ele …