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ACS Nano. 2014 Feb 25;8(2):1759-70. doi: 10.1021/nn406156b. Epub 2014 Jan 27.

MoS2/graphene composite paper for sodium-ion battery electrodes.

Author information

1
Mechanical and Nuclear Engineering Department, Kansas State University , Manhattan, Kansas 66506, United States.

Abstract

We study the synthesis and electrochemical and mechanical performance of layered free-standing papers composed of acid-exfoliated few-layer molybdenum disulfide (MoS2) and reduced graphene oxide (rGO) flakes for use as a self-standing flexible electrode in sodium-ion batteries. Synthesis was achieved through vacuum filtration of homogeneous dispersions consisting of varying weight percent of acid-treated MoS2 flakes in GO in DI water, followed by thermal reduction at elevated temperatures. The electrochemical performance of the crumpled composite paper (at 4 mg cm(-2)) was evaluated as counter electrode against pure Na foil in a half-cell configuration. The electrode showed good Na cycling ability with a stable charge capacity of approximately 230 mAh g(-1) with respect to total weight of the electrode with Coulombic efficiency reaching approximately 99%. In addition, static uniaxial tensile tests performed on crumpled composite papers showed high average strain to failure reaching approximately 2%.

PMID:
24446875
DOI:
10.1021/nn406156b

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