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Chelation-Assisted Iron-Catalyzed C-H Activations: Scope and Mechanism.
Acc Chem Res. 2024 Jan 2;57(1):10-22. doi: 10.1021/acs.accounts.3c00294. Epub 2023 Dec 20.
Acc Chem Res. 2024.
PMID: 38116619
Free PMC article.
Consequently, we developed widely applicable methods for the versatile preparation of decorated arenes and heteroarenes, providing access to benzamides, isoquinolones, pyrrolones, pyridones, phenones, indoles, and isoindolinones, among others. Most of these reactions employed …
Consequently, we developed widely applicable methods for the versatile preparation of decorated arenes and heteroarenes, providing access to …
Iron-catalyzed oxidative monoarylation of primary amines with organozinc reagents.
Nakamura Y, Ilies L, Nakamura E.
Nakamura Y, et al.
Org Lett. 2011 Nov 18;13(22):5998-6001. doi: 10.1021/ol2024357. Epub 2011 Oct 18.
Org Lett. 2011.
PMID: 22007733
The reaction of a primary zinc amide with a diorganozinc reagent gives a secondary amine in the presence of Fe(acac)(3) as a catalyst and 1,2-dichloroisobutane (DCIB) as an oxidant. Halogen groups such as F, Cl, Br, and I are tolerated well. ...
The reaction of a primary zinc amide with a diorganozinc reagent gives a secondary amine in the presence of Fe(acac)(3) as a catalyst and …
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Iron-catalyzed chemoselective ortho arylation of aryl imines by directed C-H bond activation.
Yoshikai N, Matsumoto A, Norinder J, Nakamura E.
Yoshikai N, et al.
Angew Chem Int Ed Engl. 2009;48(16):2925-8. doi: 10.1002/anie.200900454.
Angew Chem Int Ed Engl. 2009.
PMID: 19294714
The title reaction features mild and selective C-H bond activation in the presence of aryl bromide, chloride, or sulfonate groups, and 1,2-dichloroisobutane is essential to achieve such selectivity....
The title reaction features mild and selective C-H bond activation in the presence of aryl bromide, chloride, or sulfonate groups, and 1 …
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