A high-rate biological contactor process (HRBC) can be used as primary treatment instead of a clarifier to remove particulate, colloidal and soluble fractions of organic matter via biosorption plus flotation and divert it to anaerobic digestion for methane production, simultaneously reducing secondary aeration energy demand. Pilot and bench tests were conducted at a range of contact times (15-60 min) and contactor dissolved oxygen (DO) (0.2-2.0 mg/L) using waste activated sludge (WAS) from a trickling filter/solids contact (TF/SC) process in the HRBC. Biosorption performance was lowest when contact times were <30 min and unstable at DO < 0.5 mg/L. The overall average of 20% sCOD capture was similar to previous findings by others using WAS from conventional AS. The biomethane potential (BMP) of the HRBC float material can be as high as that of primary sludge (340-400 mL CH4/g VS), which is much greater than WAS. Operating the HRBC with a long contact time (>30 min) or with high DO (>1 mg/L) increases the amount of biosorption but reduces the BMP of the float. It was also found that biosorption only effectively occurs when a WAS is paired with the wastewater from the same facility.