The contribution of ¹³⁷Cs export flux from the Tone River Japan to the marine environment

The contribution of ¹³⁷Cs transport to the marine environment via the Tone River, Japan was investigated. This river has the largest discharge among rivers on the North Pacific side of eastern Japan. The sampling site was located upstream near the river mouth and dissolved and particulate ¹³⁷Cs in the river water was measured during 2014-2015, three years after the Tokyo Electric Power Corporation Fukushima Daiichi Nuclear Power Plant (FDNPP) accident. Annual fluxes of total (dissolved and particulate) ¹³⁷Cs with considering desorption of ¹³⁷Cs from riverine particles by change of salinity from the Tone River were similar in both years (78-107 × 10⁹ Bq/y), indicating that about 0.03-0.06% of the estimated total amount of ¹³⁷Cs deposited in the catchment (1.9-2.8 × 10¹⁴ Bq) was transported to the marine environment each year. Although the annual flux was about one order of magnitude lower than the daily direct discharge into the ocean from the FDNPP (800 × 10⁹ Bq/y) during the corresponding period, continuous monitoring of rivers in the southern coastal area of east Japan on the North Pacific side are needed for the effect of ¹³⁷Cs release via the rivers in the Kanto area over the long-term.