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Chem Commun (Camb). 2014 Jun 11;50(46):6094-7. doi: 10.1039/c4cc00745j.

Two-dimensional g-C(3)N(4): an ideal platform for examining facet selectivity of metal co-catalysts in photocatalysis.

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1
Hefei National Laboratory for Physical Sciences at the Microscale, Collaborative Innovation Center of Chemistry for Energy Materials, and School of Chemistry and Materials Science, University of Science & Technology of China, Hefei, 230026, P.R. China. yjxiong@ustc.edu.cn jiangj1@ustc.edu.cn.

Abstract

Two-dimensional g-C3N4 nanosheets with few-layer thickness, ensuring equivalent charge migrations to various Pd facets, provide an ideal model system for reliably examining the facet selectivity of Pd co-catalysts. It reveals that reduction of CO2 can occur better on Pd{111} facets while H2O prefers to generate H2 on Pd{100}.

PMID:
24777281
DOI:
10.1039/c4cc00745j
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