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Dalton Trans. 2013 Sep 14;42(34):12075-8. doi: 10.1039/c3dt51776d. Epub 2013 Jul 16.

Oxidative dehydrogenation of a new tetra-amine N4-donor macrocycle tunes the nickel(II) spin state from high spin to low spin.

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1
Department of Chemistry and MacDiarmid Institute for Advanced Materials and Nanotechnology, University of Otago, PO box 56, Dunedin, New Zealand.

Abstract

The nickel(II) spin state in a series of N4-donor macrocycles differing in the number of imine bonds is tuned from low spin (2 imines) to low or high spin (1 imine; non- or coordinating co-ligand) to high spin (no imines).

PMID:
23860587
DOI:
10.1039/c3dt51776d
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