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Dalton Trans. 2013 Apr 28;42(16):5607-10. doi: 10.1039/c3dt50518a.

Iron-mediated C-H bond amination by organic azides on a tripodal bis(anilido)iminophosphorane platform.

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1
State Key Laboratory of Organometallic Chemistry, Shanghai Institute of Organic Chemistry, Chinese Academy of Sciences, 345 Lingling Road, Shanghai, 200032, People's Republic of China.

Abstract

The bis(anilido)iminophosphorane complex, abbreviated as [((Mes)N2N(Ad))Fe(THF)], can react with alkyl azides to yield ligand-based C-H bond amination products suggesting the high reactivity of iron(IV)-imido species supported by the tripodal bis(anilido)iminophosphorane ligand platform [(Mes)N2N(Ad)](2-).

PMID:
23478513
DOI:
10.1039/c3dt50518a
[Indexed for MEDLINE]
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