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J Am Chem Soc. 2012 Dec 19;134(50):20326-9. doi: 10.1021/ja310981m. Epub 2012 Dec 4.

Re-mediated C-C coupling of pyridines and imidazoles.

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1
Departamento de Química Orgánica e Inorgánica-IUQOEM, Universidad de Oviedo-CSIC, C/Julián Clavería, 8, 33006 Oviedo-Spain.

Abstract

Rhenium tricarbonyl complexes with three N-heterocyclic ligands (N-alkylimidazoles or pyridines) undergo deprotonation with KN(SiMe(3))(2) and then oxidation with AgOTf to afford complexes with pyridylimidazole or bipyridine bidentate ligands resulting from deprotonation, C-C coupling and rearomatization.

PMID:
23205724
DOI:
10.1021/ja310981m
[Indexed for MEDLINE]
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