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Chem Commun (Camb). 2013 Jan 7;49(2):158-60. doi: 10.1039/c2cc37036k. Epub 2012 Nov 20.

Relaxations in heterolanthanide dinuclear single-molecule magnets.

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1
MOE Key Laboratory of Bioinorganic and Synthetic Chemistry, School of Chemistry and Chemical Engineering, Sun Yat-Sen University, Guangzhou 510275, China.

Abstract

A heterospin dinuclear complex [Dy(0.87)Yb(1.13)(H(2)cht)(2)Cl(4)(H(2)O)(MeCN)]·MeCN shows shifts of the relaxation barriers with respect to the barriers observed in homospin Dy(2) and Yb(2) isostructural complexes. The origin of slow relaxation in the latter two compounds was elucidated by ab initio calculations.

PMID:
23168878
DOI:
10.1039/c2cc37036k
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