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Chem Commun (Camb). 2009 Apr 14;(14):1843-5. doi: 10.1039/b821398d. Epub 2009 Feb 19.

Pentavalent uranyl stabilized by a dianionic bulky tetradentate ligand.

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1
Laboratoire de Reconnaissance Ionique et Chimie de Coordination, INAC, CEA-Grenoble, Grenoble Cedex 09, France.

Abstract

A pentavalent uranyl complex supported by a bulky dianionic tetradentate (ONNO)-type salan ligand has been prepared by direct synthesis from the iodide precursor {[UO(2)Py(5)][KI(2)Py(2)]}(n), and displays high stability towards disproportionation and ligand dissociation but reactivity towards oxidizing substrates.

PMID:
19319420
DOI:
10.1039/b821398d
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