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Org Lett. 2006 Oct 26;8(22):5169-71.

Asymmetric syntheses of (-)-mitorubrin and related azaphilone natural products.

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1
Department of Chemistry and Center for Chemical Methodology and Library Development, Boston University, Boston, MA 02215, USA

Abstract

Asymmetric syntheses of (-)-mitorubrin and related azaphilone natural products are reported. Key steps involve copper-mediated, enantioselective oxidative dearomatization to prepare the azaphilone core and olefin cross-metathesis for side-chain installation. [reaction: see text].

PMID:
17048870
DOI:
10.1021/ol062233m
[Indexed for MEDLINE]
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