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Proc Natl Acad Sci U S A. 2006 Jun 13;103(24):8928-33. Epub 2006 Jun 5.

Cu-catalyzed cross-dehydrogenative coupling: a versatile strategy for C-C bond formations via the oxidative activation of sp(3) C-H bonds.

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1
Department of Chemistry, McGill University, 801 Sherbrooke Street West, Montreal, QC, Canada H3A 2K6.

Abstract

Cu-catalyzed cross-dehydrogenative coupling (CDC) methodologies were developed based on the oxidative activation of sp(3) C-H bonds adjacent to a nitrogen atom. Various sp, sp(2), and sp(3) C-H bonds of pronucleophiles were used in the Cu-catalyzed CDC reactions. Based on these results, the mechanisms of the CDC reactions also are discussed.

PMID:
16754869
PMCID:
PMC1482542
DOI:
10.1073/pnas.0601687103
[Indexed for MEDLINE]
Free PMC Article
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