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Phys Rev Lett. 2005 Dec 31;95(26):267207. Epub 2005 Dec 27.

Unifying ultrafast magnetization dynamics.

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Department of Applied Physics, Center for NanoMaterials (cNM) Eindhoven University of Technology, The Netherlands.


We present a microscopic model that successfully explains the ultrafast equilibration of magnetic order in ferromagnetic metals at a time scale tau(M) of only a few hundred femtoseconds after pulsed laser excitation. It is found that tau(M) can be directly related to the so-called Gilbert damping factor sigma that describes damping of GHz precessional motion of the magnetization vector. Independent of the spin-scattering mechanism, an appealingly simple equation relating the two key parameters via the Curie temperature T(C) is derived, tau(M) approximately c(0)h/k(B)T(C)sigma, with h and k(B) the Planck and Boltzmann constants, respectively, and the prefactor c(0) approximately 1/4). We argue that phonon-mediated spin-flip scattering may contribute significantly to the sub-ps response.

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