High mobility and low density of trap states in dual-solid-gated PbS nanocrystal field-effect transistors

Adv Mater. 2015 Mar 25;27(12):2107-12. doi: 10.1002/adma.201404495. Epub 2015 Feb 17.

Abstract

Dual-gated PbS nanocrystal field-effect transistors employing SiO2 and Cytop as gate dielectrics are fabricated. The obtained electron mobility (0.2 cm(2) V(-1) s(-1) ) and the high on/off ratio (10(5) -10(6) ), show that the controlled nanocrystal assembly (obtained with self-assembled monolayers), as well as the trap density reduction (using Cytop as dielectric), are crucial steps for the future application of nanocrystals.

Keywords: ambipolar transistors; colloidal nanocrystals; density of trap states; field effect transistors.