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Chem Commun (Camb). 2014 Feb 21;50(15):1842-4. doi: 10.1039/c3cc48882a. Epub 2014 Jan 8.

Efficient photocatalytic hydrogen generation from water by a cationic cobalt(II) porphyrin.

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  • 1Dipartimento di Scienze Chimiche e Farmaceutiche, Universit√† degli Studi di Ferrara, Via Fossato di Mortara 17-19, 44121 Ferrara, Italy. mirco.natali@unife.it snf@unife.it.


Efficient photocatalytic hydrogen evolution is obtained from 1 M phosphate buffer at pH 7 in the presence of a Ru(bpy)3(2+) sensitizer, an ascorbic acid sacrificial donor, and a water-soluble Co(II) porphyrin catalyst. Spectroscopic investigation of the system by stationary and time-resolved techniques enables a complete characterization of the photoinduced dynamics.

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