Photooxidative cleavage of zinc 20-substituted chlorophyll derivatives: conformationally P-helix-favored formation of regioselectively 19-20 opened linear tetrapyrroles

Photochem Photobiol Sci. 2012 Jun;11(6):898-907. doi: 10.1039/c1pp05301a. Epub 2011 Dec 2.

Abstract

Photoreaction of zinc methyl 20-substituted meso(pyro)pheophorbide-a prepared by modifying naturally occurring chlorophyll-a in the presence of oxygen molecules gave its C19-C20 oxidative cleavage (1-carbonyl-19-oxo-bilatrienes) as the major products and the regioisomeric C1-C20 cleavage (19-carbonyl-1-oxo-bilatrienes) as the minor products. The resulting zinc complexes of linear tetrapyrroles took a helical conformation and the P-conformers were preferential over the M-stereoisomers due to the presence of their 17S,18S-chiral centers. The helical conformers (diastereomers) of the corresponding nickel complexes were separated by reverse-phase or chiral HPLC and their conformational changes were observed in solution.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Chlorophyll / analogs & derivatives
  • Chlorophyll / chemical synthesis
  • Chlorophyll / chemistry*
  • Chlorophyll A
  • Coordination Complexes / chemistry
  • Crystallography, X-Ray
  • Light
  • Molecular Conformation
  • Oxidation-Reduction
  • Stereoisomerism
  • Tetrapyrroles / chemistry*
  • Zinc / chemistry*

Substances

  • Coordination Complexes
  • Tetrapyrroles
  • Chlorophyll
  • pheophorbide a
  • Zinc
  • Chlorophyll A