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Rev Sci Instrum. 2011 Jun;82(6):063102. doi: 10.1063/1.3596453.

An efficient setup for femtosecond stimulated Raman spectroscopy.

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  • 1Department of Chemistry, Humboldt Universität zu Berlin, Brook-Taylor-Str. 2, D-12489 Berlin, Germany.


We present an efficient and robust setup for femtosecond stimulated Raman (FSR) spectroscopy with 60 fs and 10 cm(-1) resolution. Raman pulses of 0.5-5 ps are tunable between 450-750 nm with energies 1-10 μJ. Experimental features of the setup, signal processing, and data treatment are discussed in detail to be readily reproduced in other labs. The setup is tested by measuring FSR spectra of stilbene in solution.

© 2011 American Institute of Physics

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