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Phys Chem Chem Phys. 2010 Jun 28;12(24):6330-2. doi: 10.1039/b926731j. Epub 2010 Mar 17.

Hydrogen induced CO activation on open Ru and Co surfaces.

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  • 1Schuit Institute of Catalysis, Eindhoven University of Technology, P.O. Box 513, 5600 MB Eindhoven, The Netherlands. s.g.shetty@tue.nl

Abstract

An optimum reaction path for CO activation is an important issue in the Fischer-Tropsch synthesis for the production of liquid hydrocarbons from syngas. In the present theoretical study, we show that the CO activation on open Ru and Co surfaces consisting of active six-fold sites is initiated through the carbide mechanism instead of the hydrogen assisted pathway.

PMID:
20532417
[PubMed]
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