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J Phys Chem A. 2007 Sep 27;111(38):9417-23. Epub 2007 Sep 5.

Theoretical study of above-threshold dissociation on diatomic molecules by using nonresonant intense laser pulses.

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  • 1Kinjo University, Kasama, Hakusan 924-8511, Japan. sugimori@kinjo.ac.jp


The above-threshold dissociation of the ground state of a OH molecule under intense nonresonant laser pulses has been studied using the time-dependent Schrödinger equation with discrete variable representation. The applied field is assumed as a two-color mixed nonresonant laser pulses which has the nonresonant frequency omega and the overtone 2omega. After modulating the relative phase factor between the omega and 2omega pulse, we extracted a three-photon absorption peak or a five-photon absorption peak in the ATD spectrum.

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